Description (deu)
This talk was part of the Workshop on "Spin-Orbit Entangled Quantum Magnetism" held at the ESI September 23 -- 27, 2024.
The Dirac-Mott insulator 5d1 Ba2NaOsO6 (BNOO) offers an optimal playground to study the effect of the intricate interplay between electron correlations and spin-orbit (SO) coupling when their energy scales are comparable in size. As a result, this material shows local distortions from the cubic symmetry revealing the presence of a broken local point symmetry (BLPS) phase as a precursor to a canted-antiferromagnetic state driven by a multipolar order, most likely of the antiferro-quadrupolar type [1].
Here we investigate the evolution of the magnetic and BLPS phases as a function the electron charge doping induced by the Ca/Na heterovalent substitution of Ba2Na1−xCaxOsO6 in the whole 0